Jolie and Pitt have repeatedly denied reports they are a couple since Pitt and Aniston ended their marriage in January, despite numerous pictures of the Mr. and Mrs. Smith co-stars holidaying with Jolie's adopted son Maddox.
But the former Friends star admits she's still besotted with the hunk even though they are no longer on speaking terms.
She tells Vanity Fair magazine, "I will love him for the rest of my life. He's a fantastic man."
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